It sounds like the new The Pains of Being Pure at Heart album is bringing their sound up to be more loud and My Bloody Valentine-like and a slightly less indie pop. The album's title track brings some of that to life.
Look for the new album Belong new album on Mar. 15, they're working with producer Flood (Smashing Pumpkins, U2, PJ Harvey) and mixer Alan Moulder (My Bloody Valentine, The Jesus & Mary Chain, Arctic Monkeys).
Also try:
STREAM: The Pains of Being Pure at Heart - Heart In Your Heartbreak